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@ARTICLE{Mondal:154648,
author = {Mondal, Kartik Chandra and Roesky, Herbert W. and Dittrich,
Birger and Holzmann, Nicole and Hermann, Markus and
Frenking, Gernot and Meents, Alke},
title = {{F}ormation of a 1,4-{D}iamino-2,3-disila-1,3-butadiene
{D}erivative},
journal = {Journal of the American Chemical Society},
volume = {135},
number = {43},
issn = {1520-5126},
address = {Washington, DC},
publisher = {American Chemical Society},
reportid = {DESY-2013-01007},
pages = {15990 - 15993},
year = {2013},
abstract = {A 1,4-diamino-2,3-disila-1,3-butadiene derivative of
composition (Me2-cAAC)2(Si2Cl2) (Me2-cAAC =
:C(CMe2)2(CH2)N-2,6-iPr2C6H3) was synthesized by reduction
of the Me2-cAAC:SiCl4 adduct with KC8. This compound is
stable at 0 °C for 3 months in an inert atmosphere.
Theoretical studies reveal that the silicon atoms exhibit
pyramidal coordination, where the Cl–Si–Si–Cl dihedral
angle is twisted by 43.3° (calcd 45.9°). The two
silicon–carbon bonds are intermediates between single and
double Si–C bonds due to twisting of the C–Si–Si–C
dihedral angle (163.6°).},
cin = {FS-PE / DOOR},
ddc = {540},
cid = {I:(DE-H253)FS-PE-20120731 / I:(DE-H253)HAS-User-20120731},
pnm = {PETRA Beamline P11 (POF2-54G14)},
pid = {G:(DE-H253)POF2-P11-20130405},
experiment = {EXP:(DE-H253)P-P11-20150101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000326487800007},
pubmed = {pmid:24134747},
doi = {10.1021/ja4072139},
url = {https://bib-pubdb1.desy.de/record/154648},
}