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@ARTICLE{Rawolle:139000,
      author       = {Rawolle, M. and Niedermeier, M. A. and Kaune, G. and
                      Perlich, J. and Lellig, P. and Memesa, M. and Cheng, Y.-J.
                      and Gutmann, J. S. and Müller-Buschbaum, P. and DESY},
      title        = {{F}abrication and characterization of nanostructured
                      titania films with integrated function from
                      inorganic-organic hybrid materials},
      journal      = {Chemical Society reviews},
      volume       = {41},
      issn         = {0306-0012},
      address      = {London},
      publisher    = {Soc.},
      reportid     = {PHPPUBDB-23858},
      pages        = {5131-5142},
      year         = {2012},
      abstract     = {Nanostructured titania films are of growing interest due to
                      their application in future photovoltaic technologies.
                      Therefore, a lot of effort has been put into the controlled
                      fabrication and tailoring of titania nanostructures. The
                      controlled sol-gel synthesis of titania, in particular in
                      combination with block copolymer templates, is very
                      promising because of its high control on the nanostructure,
                      easy application and cheap processing possibilities. This
                      tutorial review gives a short overview of the structural
                      control of titania films gained by using templated sol-gel
                      chemistry and shows how this approach is extended by the
                      addition of further functionality to the films. Different
                      expansions of the sol-gel templating are possible by the
                      fabrication of gradient samples, by the addition of a
                      homopolymer, by the combination with micro-fluidics and also
                      by the application of novel precursors for low-temperature
                      processing. Moreover, hierarchically structured titania
                      films can be fabricated via the subsequent application of
                      several sol-gel steps or via the inclusion of colloidal
                      templates in a one-step process. Integrated function in the
                      block copolymer used in the sol-gel synthesis allows for the
                      fabrication of an integrated blocking layer or an integrated
                      hole-conductor. Both approaches grant a one-step fabrication
                      of two components of a working solar cell, which make them
                      very promising towards a cheap solar cell production route.
                      Looking to the complete solar cell, the top contact is also
                      of great importance as it influences the function of the
                      whole solar cell. Thus, the mechanisms acting in the top
                      contact formation are also reviewed. For all these aspects,
                      characterization techniques that allow for a structural
                      investigation of nanostructures inside the active layers are
                      important. Therefore, the characterization techniques that
                      are used in real space as well as in reciprocal space are
                      explained shortly as well.},
      cin          = {HASYLAB},
      ddc          = {540},
      cid          = {$I:(DE-H253)HASYLAB_-2012_-20130307$},
      pnm          = {DORIS Beamline BW4 (POF2-54G13) / FS-Proposal: II-20100012
                      (II-20100012)},
      pid          = {G:(DE-H253)POF2-BW4-20130405 / G:(DE-H253)II-20100012},
      experiment   = {EXP:(DE-H253)D-BW4-20150101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:22415549},
      UT           = {WOS:000306227900008},
      doi          = {10.1039/c2cs15321a},
      url          = {https://bib-pubdb1.desy.de/record/139000},
}