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@ARTICLE{Budewig:610668,
author = {Budewig, Laura and Son, Sang-Kil and Santra, Robin},
title = {{E}lectron-cloud alignment dynamics induced by an intense
{X}-ray free-electron laser pulse: a case study on atomic
argon},
journal = {Communications Physics},
volume = {7},
number = {1},
issn = {2399-3650},
address = {London},
publisher = {Springer Nature},
reportid = {PUBDB-2024-04674},
pages = {363},
year = {2024},
abstract = {In an intense X-ray free-electron laser (XFEL) pulse, atoms
are sequentially ionised by multiple X-ray photons.
Photoionisation generally induces an alignment of the
electron cloud of the produced atomic ion regarding its
orbital-angular-momentum projections. However, how the
alignment evolves during sequential X-ray multi-photon
ionisation accompanied by decay processes has been
unexplored. Here we present a theoretical prediction of the
time evolution of the electron-cloud alignment of argon ions
induced by XFEL pulses. To this end, we calculate
state-resolved ionisation dynamics of atomic argon
interacting with an intense linearly polarised X-ray pulse,
which generates ions in a wide range of charge states with
non-zero orbital- and spin-angular momenta. Employing
time-resolved alignment parameters, we predict the existence
of non-trivial alignment dynamics during intense XFEL
pulses. This implies that even if initially the atomic
electron cloud is perfectly spherically symmetric, X-ray
multi-photon ionisation can lead to noticeable reshaping of
the electron cloud.},
cin = {CFEL-DESYT / FS-CFEL-3},
ddc = {530},
cid = {I:(DE-H253)CFEL-DESYT-20160930 /
I:(DE-H253)FS-CFEL-3-20120731},
pnm = {631 - Matter – Dynamics, Mechanisms and Control
(POF4-631) / HIDSS-0002 - DASHH: Data Science in Hamburg -
Helmholtz Graduate School for the Structure of Matter
$(2019_IVF-HIDSS-0002)$},
pid = {G:(DE-HGF)POF4-631 / $G:(DE-HGF)2019_IVF-HIDSS-0002$},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001351613500001},
doi = {10.1038/s42005-024-01852-x},
url = {https://bib-pubdb1.desy.de/record/610668},
}