Journal Article

PUBDB-2024-00198

http://join2-wiki.gsi.de/foswiki/pub/Main/Artwork/join2_logo100x88.png Attosecond-pump attosecond-probe x-ray spectroscopy of liquid water

Li, S. ; Lu, L. ; Bhattacharyya, S.CFEL*DESY* ; Pearce, C. ; Li, K. ; Nienhuis, E. T. ; Doumy, G. ; Schaller, R. D. ; Moeller, S. ; Lin, M.-F. ; Dakovski, G. ; Hoffman, D. J. ; Garratt, D. ; Larsen, K. A. ; Koralek, J. D. ; Hampton, C. Y. ; Cesar, D. ; Duris, J. ; Zhang, Z. ; Sudar, N. ; Cryan, J. P. ; Marinelli, A. ; Li, X. (Corresponding author) ; Inhester, L.CFEL*Extern*XFEL.EU*DESY* ; Santra, R. (Corresponding author)CFEL*XFEL.EU*DESY* ; Young, L. (Corresponding author)Extern*XFEL.EU*

2024
Assoc. Washington, DC

This record in other databases:        

Please use a persistent id in citations: doi:10.1126/science.adn6059  doi:10.3204/PUBDB-2024-00198

Abstract: Attosecond-pump/attosecond-probe experiments have long been sought as the most straightforward method for observing electron dynamics in real time. Although there has been much success with overlapped near-infrared femtosecond and extreme ultraviolet attosecond pulses combined with theory, true attosecond-pump/attosecond-probe experiments have been limited. We used a synchronized attosecond x-ray pulse pair from an x-ray free-electron laser to study the electronic response to valence ionization in liquid water through all x-ray attosecond transient absorption spectroscopy (AX-ATAS). Our analysis showed that the AX-ATAS response is confined to the subfemtosecond timescale, eliminating any hydrogen atom motion and demonstrating experimentally that the 1b$_1$ splitting in the x-ray emission spectrum is related to dynamics and is not evidence of two structural motifs in ambient liquid water.

Note: ISSN 1095-9203 not unique: **3 hits**.

---

Contributing Institute(s):

1. FS-CFEL-3 (CFEL-DESYT)
2. CFEL-Theory (FS-CFEL-3)

Research Program(s):

1. 631 - Matter – Dynamics, Mechanisms and Control (POF4-631) (POF4-631)
2. AIM, DFG project G:(GEPRIS)390715994 - EXC 2056: CUI: Advanced Imaging of Matter (390715994) (390715994)

Experiment(s):

1. No specific instrument

Appears in the scientific report 2024

---

Database coverage:
; ; BIOSIS Previews ; Biological Abstracts ; Chemical Reactions ; Clarivate Analytics Master Journal List ; Current Contents - Agriculture, Biology and Environmental Sciences ; Current Contents - Life Sciences ; Current Contents - Physical, Chemical and Earth Sciences ; Ebsco Academic Search ; Essential Science Indicators ; IF >= 50 ; Index Chemicus ; JCR ; SCOPUS ; Science Citation Index Expanded ; Web of Science Core Collection ; Zoological Record

---