TY - JOUR AU - Ding, Thomas AU - Rebholz, Marc AU - Aufleger, Lennart AU - Hartmann, Maximilian AU - Stooß, Veit AU - Magunia, Alexander AU - Birk, Paul AU - Borisova, Gergana Dimitrova AU - da Costa Castanheira, Carina AU - Rupprecht, Patrick AU - Mi, Yonghao AU - Gaumnitz, Thomas AU - Loh, Zhi-Heng AU - Roling, Sebastian AU - Butz, Marco AU - Zacharias, Helmut AU - Düsterer, Stefan AU - Treusch, Rolf AU - Ott, Christian AU - Pfeifer, Thomas TI - XUV pump–XUV probe transient absorption spectroscopy at FELs JO - Faraday discussions VL - 228 SN - 1364-5498 CY - Cambridge [u.a.] PB - Soc. M1 - PUBDB-2021-02839 SP - 519 - 536 PY - 2021 AB - The emergence of ultra-intense extreme-ultraviolet (XUV) and X-ray free-electron lasers (FELs) has opened the door for the experimental realization of non-linear XUV and X-ray spectroscopy techniques. Here we demonstrate an experimental setup for an all-XUV transient absorption spectroscopy method for gas-phase targets at the FEL. The setup combines a high spectral resolving power of E/ΔE ≈ 1500 with sub-femtosecond interferometric resolution, and covers a broad XUV photon-energy range between approximately 20 and 110 eV. We demonstrate the feasibility of this setup firstly on a neon target. Here, we intensity- and time-resolve key aspects of non-linear XUV-FEL light–matter interactions, namely the non-resonant ionization dynamics and resonant coupling dynamics of bound states, including XUV-induced Stark shifts of energy levels. Secondly, we show that this setup is capable of tracking the XUV-initiated dissociation dynamics of small molecular targets (oxygen and diiodomethane) with site-specific resolution, by measuring the XUV transient absorption spectrum. In general, benefitting from a single-shot detection capability, we show that the setup and method provides single-shot phase-locked XUV pulse pairs. This lays the foundation to perform, in the future, experiments as a function of the XUV interferometric time delay and the relative phase, which enables advanced coherent non-linear spectroscopy schemes in the XUV and X-ray spectral range. LB - PUB:(DE-HGF)16 C6 - 33575691 UR - <Go to ISI:>//WOS:000664793300026 DO - DOI:10.1039/D0FD00107D UR - https://bib-pubdb1.desy.de/record/459956 ER -