Home > Private Collections > >MPG > MPSD > Tailored Pump-Probe Transient Spectroscopy With Time-Dependent Density-Functional Theory: Controlling Absorption Spectra > print

001     307553
005     20211110134858.0
024 7 _ |a 10.1140/epjb/e2016-70064-0
|2 doi
024 7 _ |a 1434-6028
|2 ISSN
024 7 _ |a 1434-6036
|2 ISSN
037 _ _ |a PUBDB-2016-03264
041 _ _ |a English
082 _ _ |a 530
100 1 _ |a Walkenhorst, Jessica
|0 P:(DE-HGF)0
|b 0
|e Corresponding author
245 _ _ |a Tailored Pump-Probe Transient Spectroscopy With Time-Dependent Density-Functional Theory: Controlling Absorption Spectra
260 _ _ |a Berlin
|c 2016
|b Springer
336 7 _ |a article
|2 DRIVER
336 7 _ |a Output Types/Journal article
|2 DataCite
336 7 _ |a Journal Article
|b journal
|m journal
|0 PUB:(DE-HGF)16
|s 1480588388_17216
|2 PUB:(DE-HGF)
336 7 _ |a ARTICLE
|2 BibTeX
336 7 _ |a JOURNAL_ARTICLE
|2 ORCID
336 7 _ |a Journal Article
|0 0
|2 EndNote
500 _ _ |a (c) EDP Sciences, Societa Italiana di Fisica, Springer-Verlag. Post referee full text in progress (embargo 1 year from 15.05.2016).
520 _ _ |a Recent advances in laser technology allow us to follow electronic motion at its natural time-scale with ultra-fast time resolution, leading the way towards attosecond physics experiments of extreme precision. In this work, we assess the use of tailored pumps in order to enhance (or reduce) some given features of the probe absorption (for example, absorption in the visible range of otherwise transparent samples). This type of manipulation of the system response could be helpful for its full characterization, since it would allow us to visualize transitions that are dark when using unshaped pulses. In order to investigate these possibilities, we perform first a theoretical analysis of the nmon-equilibrium response function in this context, aided by one simple numerical model of the hydrogen atom. Then, we proceed to investigate the feasibility of using time-dependent density-functional theory as a means to implement, theoretically, this absorption-optimization idea, for more complex atoms or molecules. We conclude that the proposed idea could in principle be brought to the laboratory: tailored pump pulses can excite systems into light-absorbing states. However, we also highlight the severe numerical and theoretical difficulties posed by the problem: large-scale non-equilibrium quantum dynamics are cumbersome, even with TDDFT, and the shortcomingsof state-of-the-art TDDFT functionals may still be serious for these out-of-equilibrium situations.
588 _ _ |a Dataset connected to CrossRef
693 _ _ |0 EXP:(DE-MLZ)NOSPEC-20140101
|5 EXP:(DE-MLZ)NOSPEC-20140101
|e No specific instrument
|x 0
700 1 _ |a De Giovannini, Umberto
|0 P:(DE-HGF)0
|b 1
700 1 _ |a Castro, Alberto
|0 P:(DE-HGF)0
|b 2
700 1 _ |a Rubio, Angel
|0 P:(DE-H253)PIP1023770
|b 3
773 _ _ |a 10.1140/epjb/e2016-70064-0
|g Vol. 89, no. 5, p. 128
|0 PERI:(DE-600)1459068-2
|n 5
|p 128
|t The @European physical journal / B
|v 89
|y 2016
|x 1434-6036
856 4 _ |u https://bib-pubdb1.desy.de/record/307553/files/10.1140_epjb_e2016-70064-0.pdf
|y Restricted
856 4 _ |u https://bib-pubdb1.desy.de/record/307553/files/10.1140_epjb_e2016-70064-0.gif?subformat=icon
|x icon
|y Restricted
856 4 _ |u https://bib-pubdb1.desy.de/record/307553/files/10.1140_epjb_e2016-70064-0.jpg?subformat=icon-1440
|x icon-1440
|y Restricted
856 4 _ |u https://bib-pubdb1.desy.de/record/307553/files/10.1140_epjb_e2016-70064-0.jpg?subformat=icon-180
|x icon-180
|y Restricted
856 4 _ |u https://bib-pubdb1.desy.de/record/307553/files/10.1140_epjb_e2016-70064-0.jpg?subformat=icon-640
|x icon-640
|y Restricted
856 4 _ |u https://bib-pubdb1.desy.de/record/307553/files/10.1140_epjb_e2016-70064-0.pdf?subformat=pdfa
|x pdfa
|y Restricted
856 4 _ |u https://bib-pubdb1.desy.de/record/307553/files/1601.04544v1.pdf
|y Restricted
|z StatID:(DE-HGF)0510
856 4 _ |u https://bib-pubdb1.desy.de/record/307553/files/1601.04544v1.gif?subformat=icon
|x icon
|y Restricted
|z StatID:(DE-HGF)0510
856 4 _ |u https://bib-pubdb1.desy.de/record/307553/files/1601.04544v1.jpg?subformat=icon-1440
|x icon-1440
|y Restricted
|z StatID:(DE-HGF)0510
856 4 _ |u https://bib-pubdb1.desy.de/record/307553/files/1601.04544v1.jpg?subformat=icon-180
|x icon-180
|y Restricted
|z StatID:(DE-HGF)0510
856 4 _ |u https://bib-pubdb1.desy.de/record/307553/files/1601.04544v1.jpg?subformat=icon-640
|x icon-640
|y Restricted
|z StatID:(DE-HGF)0510
856 4 _ |u https://bib-pubdb1.desy.de/record/307553/files/1601.04544v1.pdf?subformat=pdfa
|x pdfa
|y Restricted
|z StatID:(DE-HGF)0510
909 C O |o oai:bib-pubdb1.desy.de:307553
|q driver
910 1 _ |a Centre for Free-Electron Laser Science
|0 I:(DE-H253)_CFEL-20120731
|k CFEL
|b 3
|6 P:(DE-H253)PIP1023770
910 1 _ |a Max-Planck-Gesellschaft zur Förderung der Wissenschaften
|0 I:(DE-588b)2019024-4
|k MPG
|b 3
|6 P:(DE-H253)PIP1023770
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)0200
|2 StatID
|b SCOPUS
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)0600
|2 StatID
|b Ebsco Academic Search
915 _ _ |a JCR
|0 StatID:(DE-HGF)0100
|2 StatID
|b EUR PHYS J B : 2015
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)0150
|2 StatID
|b Web of Science Core Collection
915 _ _ |a WoS
|0 StatID:(DE-HGF)0110
|2 StatID
|b Science Citation Index
915 _ _ |a WoS
|0 StatID:(DE-HGF)0111
|2 StatID
|b Science Citation Index Expanded
915 _ _ |a IF < 5
|0 StatID:(DE-HGF)9900
|2 StatID
915 _ _ |a OpenAccess
|0 StatID:(DE-HGF)0510
|2 StatID
915 _ _ |a Peer Review
|0 StatID:(DE-HGF)0030
|2 StatID
|b ASC
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)1150
|2 StatID
|b Current Contents - Physical, Chemical and Earth Sciences
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)0300
|2 StatID
|b Medline
915 _ _ |a Nationallizenz
|0 StatID:(DE-HGF)0420
|2 StatID
915 _ _ |a DBCoverage
|0 StatID:(DE-HGF)0199
|2 StatID
|b Thomson Reuters Master Journal List
980 _ _ |a journal
980 _ _ |a I:(DE-H253)MPSD-20120731
980 _ _ |a I:(DE-H253)L-20120731
980 1 _ |a EXTERN4VITA

LibraryCollectionCLSMajorCLSMinorLanguageAuthor
Marc 21