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2019-05-14
14:52
[PUBDB-2019-02274] Lecture
et al
Molecular and Ultrafast Science Seminar (MUSS)
Lecture at Universität Hamburg (Hamburg, Germany), 1 Apr 2019 - 13 Jul 20192019-04-012019-07-13
CFEL Molecular and Ultrafast Science Seminar (MUSS) series. This is a general topical seminar series on developments in modern molecular and ultrafast science jointly organized by the CFEL Controlled Molecule Imaging group, the Spectroscopy of molecular processes group, the CFEL Attosecond Science group, and the CFEL Ultrafast Optics group. [...]
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2019-05-14
14:03
[PUBDB-2019-02269] Lecture
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CFEL Molecular and Ultrafast Science Seminar (MUSS)
Lecture at Universität Hamburg (), 15 Oct 2018 - 2 Feb 20192018-10-152019-02-02
CFEL Molecular and Ultrafast Science Seminar (MUSS) series. This is a general topical seminar series on developments in modern molecular physics organized by the CFEL Controlled Molecule Imaging group, the Spectroscopy of molecular processes group, the CFEL Attosecond Science group, and the CFEL Ultrafast Optics group. [...]
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2019-05-14
13:52
[PUBDB-2019-02268] Lecture/Internal Report

Seminar zur Molekülphysik / Molecular Physics Seminar
Lecture at Universität Hamburg (), 3 Apr 2018 - 16 Jul 20182018-04-032018-07-16
CFEL Molecular Physics seminar series. This is a general topical seminar series on developments in modern molecular physics organized by the CFEL-CMI group Controlled Molecule Imaging and the CFEL-MPSD group Structure and Dynamics of Cold and Controlled Molecules. [...]
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2019-04-16
14:40
[PUBDB-2019-01960] Journal Article
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Rotational Signatures of Dispersive Stacking in the Formation of Aromatic Dimers
Angewandte Chemie 131(10), 3140 - 3145 () [10.1002/ange.201812556]  GO
The aggregation of aromatic species is dictated by inter‐ and intramolecular forces. Not only is characterizing these forces in aromatic growth important for understanding grain formation in the interstellar medium, but it is also imperative to comprehend biological functions. [...]
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2019-01-28
15:11
Embargoed OpenAccess [PUBDB-2019-00819] Journal Article
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Microwave spectra and nuclear quadrupole structure of the $NH_{3}–N_{2}$ van der Waals complex and its deuterated isotopologues
The microwave spectrum of the NH$_3$–N$_2$ van der Waals complex has been observed in a supersonic molecular jet expansion via broadband (2-8 GHz) chirped-pulse Fourier-transform microwave spectroscopy. Two pure rotational R(0) transitions (J = 1 − 0) with different hyperfine structure patterns were detected. [...]
Published on 2018-12-11. Available in OpenAccess from 2019-12-11.: Download fulltextPDF Download fulltextPDF (PDFA);
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2019-01-28
13:47
[PUBDB-2019-00792] Journal Article
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State-Specific Enrichment of Chiral Conformers with Microwave Spectroscopy
An interesting class of molecules is that in which the molecules do not possess a stereogenic center but can become chiral because of their spatial arrangement. These molecules can be seen as chiral conformers, whose two nonsuperimposable forms can interconvert from one to another by rotations about single bonds. [...]
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2019-01-28
13:40
[PUBDB-2019-00790] Journal Article

Sensing Chirality with Rotational Spectroscopy
Chiroptical spectroscopy techniques for the differentiation of enantiomers in the condensed phase are based on an established paradigm that relies on symmetry breaking using circularly polarized light. We review a novel approach for the study of chiral molecules in the gas phase using broadband rotational spectroscopy, namely microwave three-wave mixing, which is a coherent, nonlinear, and resonant process. [...]
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2019-01-11
14:10
Embargoed OpenAccess [PUBDB-2019-00407] Journal Article

Electron-withdrawing effects on the molecular structure of 2- and 3-nitrobenzonitrile revealed by broadband rotational spectroscopy and their comparison with 4-nitrobenzonitrile
The rotational spectra of 2- and 3-nitrobenzonitrile were recorded via chirped-pulse Fourier transform microwave spectroscopy in the frequency range of 2–8 GHz. These molecules each display large dipole moments, making them viable candidates for deceleration and trapping experiments with AC-electric fields. [...]
Published on 2018-08-03. Available in OpenAccess from 2019-08-03.: Nitroanisole - Download fulltextPDF Download fulltextPDF (PDFA); Supplementary_material - Download fulltextPDF Download fulltextPDF (PDFA); Restricted: Download fulltextPDF Download fulltextPDF (PDFA);
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2019-01-11
08:51
[PUBDB-2019-00384] Journal Article
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The Effect of Dispersion on the Structure of Diphenyl Ether Aggregates
Dispersion interactions can play an important role in understanding unusual binding behaviors. This is illustrated by a systematic study of the structural preferences of diphenyl ether (DPE)–alcohol aggregates, for which OH⋅⋅⋅O‐bound or OH⋅⋅⋅$π$‐bound isomers can be formed. [...]
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2019-01-11
08:26
Embargoed OpenAccess [PUBDB-2019-00379] Journal Article

Flexibility at the Fringes: Conformations of the Steroid Hormone $\beta$-Estradiol
ChemPhysChem 19(21), 2915 - 2920 () [10.1002/cphc.201800647]  GO
We present the accurate experimental structure of the steroid hormone β‐estradiol obtained with high‐resolution rotational spectroscopy under the solvent free, isolated, and cold conditions of a molecular jet. This is the first time that the rotational signature of a steroid hormone is reported. [...]
Published on 2018-11-06. Available in OpenAccess from 2019-11-06.: TOC - Download fulltextPDF Download fulltextPDF (PDFA); Estradiol_manuscript - Download fulltextPDF Download fulltextPDF (PDFA); Estradiol_supporting_information - Download fulltextPDF Download fulltextPDF (PDFA); Restricted: Download fulltextPDF Download fulltextPDF (PDFA);
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